Robust photo-induced pure spin current in graphene–graphane superlattices

The photogalvanic effect has been demonstrated to be an effective method to generate pure spin current. However, obtaining robust pure spin current remains a big challenge as most of the photo-induced pure spin current is dependent on the light polarization/phase angle, photon energies, or the spin alignment of electrodes. In this paper, we present a scheme for obtaining robust pure spin current in zigzag graphene–graphane superlattices (ZGSLs). Through systemic first-principles calculations, we demonstrate that robust generation of pure spin current can occur in ZGSLs with varying widths due to the centrosymmetry of the system's geometric structure and the antiferromagnetic magnetic features. Moreover, the generation of pure spin current does not depend on the photon energy or the polarization/phase angles for both linearly and elliptically polarized light, exhibiting very strong robustness. Our study suggests that ZGSLs could be highly promising candidates for practically realizing pure spin current in spintronics experiments, which presents an avenue for using graphene and its derivatives in advanced electronic devices. Furthermore, considering the experimental advancements in graphene and graphene-like materials, our investigation presents a universally applicable methodology for the generation of robust pure spin currents within low-dimensional graphene-like systems.