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We present an investigation of the computational requirements for the pseudopotential plane-wave method as a function of the number of atoms per unit cell. For systems containing a large number of atoms the computational load can be reduced if the pseudopotential operator is of a suitable form, such that it can be efficiently calculated in the position representation. The pseudopotentials examined here include local pseudopotentials, position-dependent electron-mass pseudopotentials, and separable nonlocal pseudopotentials.
Troullier et al. (Mon,) studied this question.