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Lead-halide perovskite light-emitting diodes (PeLEDs) are intrinsically capable of delivering high efficiency at high current densities compared to conventional solution-processed light-emitting diodes. While such performance and relevant high radiance have been well demonstrated in green and near-infrared ones, blue PeLEDs have lagged far behind due to extremely severe luminance-efficiency roll-off, especially in the pure-blue region (-2 (478 nm, at a CIEy coordinate below 0.15). We also achieve a high brightness reaching ∼140 000 cd m-2 under pulsed driven. Our study not only provides a useful guidance for developing bright blue PeLEDs but also resolves a long-standing puzzle regarding the interfacial properties of PACs and their impact on hole transport, and it helps with the further design of these materials for lead-halide perovskite applications.
Luo et al. (Mon,) studied this question.