The Origin and Promise of Transition Metal Dichalcogenide-Hosted Single-Photon Emitters for Quantum Technologies

Single-photon emitters (SPEs) are integral parts of several quantum technology implementations. Over the past decade or so, monolayers of transition metal dichalcogenides (TMDCs) have emerged as promising candidates for SPE platforms with attractive characteristics. To move ahead, it is necessary to understand the atomistic origin of SPEs in TMDCs─a topic that is highly debated with contradicting proposals. In this work, we critically review these existing proposals to elucidate their origin. Further, we perform a critical trend analysis for different figures of merit of TMDC-based SPEs, and we propose a characterization methodology to streamline the reporting process. Finally, we review several quantum technology implementations, where solid-state SPEs are being used, and identify the advancements required in TMDC-based SPEs for their successful adoption in these technologies.