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We present a formalism for the calculation of the optical response of semiconductors in the independent-particle approximation. The unphysical divergences at zero frequency that plagued earlier approaches are eliminated by a careful treatment of interband and intraband motion, yet the calculations can be made in a way very analogous to usual perturbation theory. The general formalism is illustrated by deriving an expression for the response coefficient for second-harmonic generation.
Sipe et al. (Fri,) studied this question.
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