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A simple dynamical criterion for crystallization of a colloidal fluid which undergoes Brownian motion is proposed, similar in spirit to the classic Lindemann melting rule. It states that the ratio of the long-time and short-time self-diffusion coefficients is a universal number very close to 0.1 along the freezing line. This phenomenological crystallization rule is confirmed both by Brownian dynamics simulations of a Yukawa liquid and by forced Rayleigh scattering experiments on charge-stabilized colloidal suspensions.
Löwen et al. (Mon,) studied this question.
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