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A Lorentzian Lie group is a Lie group endowed with a left invariant Lorentzian metric. We study left-invariant Codazzi tensors on Lorentzian Lie groups. We obtain new results on left-invariant Lorentzian metrics with harmonic curvature and non-parallel Ricci operator. In contrast to the Riemannian case, the Ricci operator of a let-invariant Lorentzian metric can be of four types: diagonal, of type \n-2, zz\, of type \n, a2\ and of type \n, a3\. We first describe Lorentzian Lie algebras with a non-diagonal Codazzi operator and with these descriptions in mind, we study three classes of Lorentzian Lie groups with harmonic curvature. Namely, we give a complete description of the Lie algebra of Lorentzian Lie groups having harmonic curvature and where the Ricci operator is non-diagonal and its diagonal part consists of one real eigenvalue.
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