Determining Key Local Vibrations in the Relaxation of Molecular Spin Qubits and Single-Molecule Magnets

= 1,2-dicyanoethylene-1,2-dithiolate), a highly coherent complex. By theoretically identifying the most relevant vibrational modes, we are able to offer general strategies to chemically design more resilient magnetic molecules, where the energy of the spin states is not coupled to vibrations.