The research aims to understand how various adsorptions contribute to effective urea electrosynthesis.
Utilized in-situ Raman spectroscopy to observe adsorptions.
Conducted ICOHP theoretical calculations to analyze interactions.
Investigated the adsorption of CO2, NO3-, and H+ on relevant substrates.
Found that the combined adsorption of CO2, NO3-, and H+ significantly enhances urea production.
Demonstrated a robust performance in urea electrosynthesis due to synergistic effects.
Abstract
The adsorptions of CO2 on Cu(0), NO3- on Cu(I) and H+ on S atoms revealed by in-situ Raman spectroscopy and ICOHP theoretical calculation, synergistically contribute to a robust urea electrosynthesis...