リチウム–硫黄電池におけるLi2S沈殿のメカニズムと動力学

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Abstract

リチウム–硫黄電池における炭素へのLi2S電極沈着の動力学が特徴づけられています。電極沈着は、電解質溶媒に強く依存する速さ定数を持つ2D ニucleation および成長プロセスによって支配されることが分かりました。成核には成長よりも大きな過剰電圧が必要であり、その結果、放電速度に依存する形態が得られます。

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Frank Y. Fan

Massachusetts Institute of Technology

W. Craig Carter

Massachusetts Institute of Technology

Yet‐Ming Chiang

National Taipei University of Technology

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Massachusetts Institute of Technology

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Fan et al. (Mon,) はこの問題を研究しました。

synapsesocial.com/papers/69c68e302ac106bc17e5be49 — DOI: https://doi.org/10.1002/adma.201501559

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Kinetics of Phase Change. II Transformation-Time Relations for Random Distribution of Nuclei· 1940 · 8,620 citations
Electrochemical nucleation· 1982 · 638 citations
Kinetics of the electrocrystallization of thin films of calomel· 1962 · 432 citations
Influence of Nonaqueous Solvents on the Electrochemistry of Oxygen in the Rechargeable Lithium−Air Battery· 2010 · 970 citations
Sulfur Speciation in Li–S Batteries Determined by Operando X-ray Absorption Spectroscopy· 2013 · 536 citations

Also consider

Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

Kinetics of Phase Change. II Transformation-Time Relations for Random Distribution of Nuclei· 1940 · 8,620 citations
Electrochemical nucleation· 1982 · 638 citations
Kinetics of the electrocrystallization of thin films of calomel· 1962 · 432 citations
Influence of Nonaqueous Solvents on the Electrochemistry of Oxygen in the Rechargeable Lithium−Air Battery· 2010 · 970 citations
Sulfur Speciation in Li–S Batteries Determined by Operando X-ray Absorption Spectroscopy· 2013 · 536 citations

リチウム–硫黄電池におけるLi2S沈殿のメカニズムと動力学

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