To explore the enhancement of solar energy conversion through improved mass transfer and exciton dissociation in nanoscale COFs.
Utilized nanoscale covalent organic frameworks (COFs) as photocatalysts.
Analyzed the pathways for proton-electron transfer and their coupling efficiency in photosynthesis.
Measured the efficiency of H2O2 production under solar irradiation.
Established a paradigm for synergistic mass transfer and exciton dissociation.
Demonstrated improved efficiency in H2O2 production compared to traditional methods.
Revealed potential for broader applications in solar energy conversion.
Abstract
ORR pathway. This work establishes a generalizable paradigm for orchestrating coupled proton-electron transfer in porous photocatalysts for efficient solar energy conversion.