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Phosphonochalcogenide-catalyzed chalcogen bonding provides enhanced stereoselectivity and reactivity in aryl-C-glycosylations compared to halogen bonding by shifting the reaction mechanism toward the SN1 domain via differentiated activation of a key bicyclic intermediate. Novelty: ClaimNovelty.NOVEL_FINDING. Consensus alignment: ConsensusAlignment.NEUTRAL.

Enhanced Selectivity of Chalcogen Bonding over Halogen Bonding Catalyzed C ‐glycosylation Through Differentiated Intermediate Activation

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