Spatially Directed Charge Transfer in a Polymer Framework for Efficient Photocatalytic Overall Water Splitting

Key Points

• The aim is to enhance the efficiency of hydrogen production through photocatalytic overall water splitting.
• Developed a polymer framework for photocatalytic reactions.
• Conducted experiments to measure hydrogen production rates under solar irradiation.
• Analyzed charge transfer mechanisms within the framework.
• Achieved hydrogen production rates exceeding 1 mmol h -1.
• Demonstrated improved charge transfer efficiency in the system.
• Provided insights on spatial arrangement impacting photocatalytic activity.