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A new nonlinear optical crystal CsLiB6O10 (CLBO), is described that can be grown from either stoichiometric melt or from solution. A large, high quality single crystal with dimensions of 14×11×11 cm3 was obtained by the top-seeded Kyropoulos method. Fourth harmonic and fifth harmonic generations of the 1.064 μm Nd:YAG laser radiation with type-I phase matching were realized in the CLBO crystal. Output pulse energies obtained were 110 mJ at 266 nm and 35 mJ at 213 nm.
Mori et al. (Mon,) studied this question.