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The chemisorption of hydrogen on metals is treated by a self-consistent calculation. Three-dimensional charge densities, interaction energies, and dipole moments are given as a function of position of the hydrogen adatoms. The results are compared with experiment. The experimental picture of a dissociated adsorbate of small dipole moment is substantiated, and the calculations are consistent with the observation that hydrogen field desorbs together with the surface atoms of the substrate.
Smith et al. (Mon,) studied this question.