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The Stokes–Einstein and Stokes–Einstein–Debye relations hold well in nonsupercooled liquids; however, sizeable deviations from the former appear in supercooled liquids, leading to a ‘‘decoupling’’ of translational diffusion from viscosity and reorientational relaxation. We attribute this breakdown and this ‘‘decoupling’’ to the existence of structured domains in the supercooled liquid.
Tarjus et al. (Tue,) studied this question.
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