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T-shaped arrangements in the homodimers A and C of benzene and hexafluorobenzene, respectively, are rationalized by polar effects, but face-to-face stacking dominates in the 1:1 heterodimer B. The dynamics of a series of fluorinated 1,8-diarylnaphthalenes clearly demonstrate the dependence of arene–arene interactions on the electronic characteristics of the arenes. The results are important for the design of supramolecular structures.
Cozzi et al. (Mon,) studied this question.
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