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We have determined the angular and velocity distributions of the CO2 product of the interaction of gas-phase O atoms with CO adsorbed on Pt(111) at 90 K. The desorption intensity is found to be strongly peaked along the surface normal, falling approximately as cos12 θf with increasing final angle, θf. The velocity distributions are found to be highly non-Boltzmann with mean energies of ∼0.6 eV, decreasing slightly with increasing θf.
Mullins et al. (Sun,) studied this question.
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