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Using the method of Doppler-free double resonance polarization spectroscopy transitions from selectively pumped levels (v′, J′) of the D1Σ+u state down to levels (v″, J″) of the X 1Σ+g state with v″= 0–140 have been measured with high accuracy. A long range analysis, based on 21 outer turning points of the IPA potential with v″=110-130 and on calculated exchange energies and second order van der Waals coefficients Cn with n=6, 8, 10, and 12 leads to a dissociation energy De =3649.5±0.8 cm−1 (0.452 49 eV). The influence of the third order C11 contribution and the hyperfine structure on the correct value of De are briefly discussed.
Weickenmeier et al. (Sat,) studied this question.
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