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Magnetic ordering in nanosized (100 and 1500 nm) nickel oxide NiO powders, prepared by the plasma synthesis method, was studied using Raman scattering spectroscopy in a wide range of temperatures from 10 to 300 K. It was observed that the intensity of two-magnon band decreases rapidly for smaller crystallites size. This effect is attributed to a decrease of antiferromagnetic spin correlations and leads to the antiferromagnetic-to-paramagnetic phase transition.
Миронова-Улмане et al. (Sat,) studied this question.
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