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This work reports the first structure-properties relationship study of ortho 2,1-c-, meta 1,2-a-, and para 1,2-bdihydroindenofluorenes, highlighting the influence of bridge rigidification on the electronic properties. This study has made it possible to devise an extended π-conjugated molecule with both a high triplet state energy level and excellent thermal and morphological stability. As a proof of concept, dihydroindenofluorenes were used as the host in sky-blue phosphorescent organic light-emitting diodes (PhOLEDs) with high performance.
Romain et al. (Tue,) studied this question.
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