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Isolated single-atom platinum (Pt) embedded in the sub-nanoporosity of 2D g-C3 N4 as a new form of co-catalyst is reported. The highly stable single-atom co-catalyst maximizes the atom efficiency and alters the surface trap states of g-C3 N4 , leading to significantly enhanced photocatalytic H2 evolution activity, 8.6 times higher than that of Pt nanoparticles and up to 50 times that for bare g-C3 N4 .
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Xiaogang Li
Shandong University
Wentuan Bi
Anhui University of Science and Technology
Lei Zhang
Guangdong Academy of Sciences
Advanced Materials
University of Science and Technology of China
Collaborative Innovation Center of Chemistry for Energy Materials
National Synchrotron Radiation Laboratory
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Li et al. (Fri,) studied this question.
synapsesocial.com/papers/69d7c7d7319e71454dbed9f4 — DOI: https://doi.org/10.1002/adma.201505281