Simultaneous Inverse Design of Materials and Structures via Deep Learning: Demonstration of Dipole Resonance Engineering Using Core–Shell Nanoparticles

Recent introduction of data-driven approaches based on deep-learning technology has revolutionized the field of nanophotonics by allowing efficient inverse design methods. In this paper, a simultaneous inverse design of materials and structure parameters of core-shell nanoparticles is achieved for the first time using deep learning of a neural network. A neural network to learn the correlation between the extinction spectra of electric and magnetic dipoles and core-shell nanoparticle designs, which include material information and shell thicknesses, is developed and trained. We demonstrate deep-learning-assisted inverse design of core-shell nanoparticles for (1) spectral tuning electric dipole resonances, (2) finding spectrally isolated pure magnetic dipole resonances, and (3) finding spectrally overlapped electric dipole and magnetic dipole resonances. Our finding paves the way for the rapid development of nanophotonics by allowing a practical utilization of deep-learning technology for nanophotonic inverse design.