Hydrogen Bonding in Self-Healing Elastomers

In the past decade, the self-healing elastomers based on multiple hydrogen bonding have attracted ample attention due to their rich chemical structures, adjustable mechanical properties, fast healing speed, and high healing efficiency. Through prolonging the service life and fast recovery of the mechanical properties, self-healing elastomers can be potentially applied in the field of wearable electronics, electronic skins, motion tracking, and health monitoring. In this perspective, we will introduce the concept and classification of self-healing materials first, then the hydrogen bonds, and the corresponding position of hydrogen-bonding units in the polymer structures. We will also conclude the potential application of hydrogen bonding-based elastomers. Finally, a summary and outlook will be provided.