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This study measured the pollution characteristics and ecological and health risks of 19 herbicides found in drinking water sources and their inflowing rivers. The targeted herbicides were prevalent in the study area, but most concentrations were well below 10 ng L-1. Acetochlor and atrazine were the dominant herbicides, although their levels were much lower than previously reported. Total herbicide residual levels were greater in April than in December and increased from upstream to downstream, resulting in the highest pollution levels found in the reservoirs, likely due to herbicides delivered from upstream and dense agricultural planting in the surrounding areas. Only atrazine and ametryn presented moderate ecological risks, while the summed risk quotients (ΣRQs) of each sample were >0.1, indicated that the total herbicide levels represented a moderate risk in all samples. For the human health risks, the risk quotients (RQ) of all target herbicides, the total RQs of each sample, and estimated life-stage RQs were far smaller than the 0.2 threshold, indicating the absence of human health risks when the water was consumed at any stage of life. However, early life stages exhibited 3-6 times higher RQ values than adulthood and should not be overlooked. And crucially, the synergistic or antagonistic effects of mixed herbicides are not well understood, and further research is needed to understand the impact of these herbicides on the ecosystem and human health, particularly possible affects in early life stages, such as infants and children.
Li et al. (2023) studied this question.