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Cluster algebras *with coefficients* are important since they appear in nature as coordinate algebras of varieties like Grassmannians, double Bruhat cells, unipotent cells, ... . The approach of Geiss-Leclerc-Schröer often yields Frobenius exact categories which allow to categorify such cluster algebras. In previous work, the third-named author has constructed Higgs categories and relative cluster categories in the relative Jacobi-finite setting (arXiv:2109.03707). Higgs categories generalize the Frobenius categories used by Geiss-Leclerc-Schröer. In this article, we construct the Higgs category and the relative cluster category in the relative Jacobi-infinite setting under suitable hypotheses. These cover for example the case of Jensen-King-Su's Grassmannian cluster category. As in the relative Jacobi-finite case, the Higgs category is no longer exact but still extriangulated in the sense of Nakaoka-Palu. We also construct a cluster character refining Plamondon's. In the appendix, Chris Fraser and the second-named author categorify quasi-cluster morphisms using Frobenius categories. A recent application of this result is due to Matthew Pressland, who uses it to prove a conjecture by Muller-Speyer.
Fraser et al. (Sun,) studied this question.