Cryogenic carbon capture design through CO2 anti-sublimation for a gas turbine exhaust: Environmental, economic, energy, and exergy analysis

To achieve a net zero-emission society, current industries must transition to become less carbon-intensive while fulfilling the rising power demand. In this study, we present a novel multigeneration system that produces power, cooling, and solid carbon dioxide by applying cryogenic carbon capture to a gas turbine flue gas. The energy recovery concept is efficiently employed to avoid energy and exergy losses in the system. The system is simulated in Aspen Plus with the mathematical models of the exergy streams and solid-vapor equilibrium written in Matlab. The performance of the plant is assessed based on energy, exergy, economic, and environmental evaluations. Thermodynamic analysis indicates that 1.2 MJ of electricity is required to capture 1 kg of CO2 from the gas turbine exhaust gas (which is lower compared to conventional systems) with 100 % CO2 purity. The net generated power, energy efficiency, exergy efficiency, m˙CO2,captured, and m˙CO2,emitted for the proposed system are 179.4 MW, 41.2 %, 59.3 %, 500,000 tons annually, and 255,000 tons a year, respectively. Sensitivity analysis shows that reducing the flue gas temperature positively impacts the CO2 content in the flue gas while having a negative effect on energy and exergy efficiency. The economic investigation shows that the system is economically profitable.