Breaking the Saturation of Sensitivity for Ultrawide Range Flexible Pressure Sensors by Soft‐Strain Effect

Abstract The flexible pressure sensors with a broad pressure range and unsaturated sensitivity are highly desired in practical applications. However, pressure sensors by piezoresistive effect are always limited by the compressibility of sensing layers, resulting in a theoretically decreasing sensitivity of less than 100%. Here, a unique strategy is proposed that utilizes the strain effect, simultaneously achieving a trade‐off between a wider pressure detection range and unsaturated sensitivity. Ascribed to the strain effect of sensing layers induced by interlaced microdomes, the sensors possess an increased sensitivity (5.22–70 MPa −1 ) over an ultrawide pressure range (45 Pa–4.1 MPa), a high‐pressure resolution (5 Pa), fast response/recovery time (30/45 ms), and a robust response under a high‐pressure loading of 3.5 MPa for more than 5000 cycles. These superior sensing performances allow the sensor to monitor large pressure. The flexible pressure sensor array can assist doctors in restoring the neutral mechanical axis, tracking knee flexion angles, and extracting gait features. Moreover, the flexible sensing array can be integrated into the joint motion surveillance system to map the balance medial–lateral contact forces on the metal compartments in real time, demonstrating the potential for further development into precise medical human–machine interfaces during total knee replacement surgery.