Emerging Liquid‐Based Memristive Devices for Neuromorphic Computation

To mimic the neural functions of the human brain, developing hardware with natural similarities to the human nervous system is crucial for realizing neuromorphic computing architectures. Owing to their capability to emulate artificial neurons and synapses, memristors are widely regarded as a leading candidate for achieving neuromorphic computing. However, most current memristor devices are solid-state. In contrast, biological nervous systems operate within an aqueous environment, and the human brain accomplishes intelligent behaviors such as information generation, transmission, and memory by regulating ion transport in neuronal cells. To achieve computing systems that are more analogous to biological systems and more energy-efficient, memristor devices based on liquid environments are developed. In contrast to traditional solid-state memristors, liquid-based memristors possess advantages such as anti-interference, low energy consumption, and low heat generation. Simultaneously, they demonstrate excellent biocompatibility, rendering them an ideal option for the next generation of artificial intelligence systems. Numerous experimental demonstrations of liquid-based memristors are reported, showcasing their unique memristive properties and novel neuromorphic functionalities. This review focuses on the recent developments in liquid-based memristors, discussing their operating mechanisms, structures, and functional characteristics. Additionally, the potential applications and development directions of liquid-based memristors in neuromorphic computing systems are proposed.