Introduction In the 21st century, self-regulated learning (SRL) plays a vital role in the cultivation of high-quality talent. Grounded in self-regulated learning theory and attachment theory, this study aims to systematically examine the relationship between adolescents’ SRL and academic achievement, considering the roles of academic emotions and teacher–student relationships (TSR). Additionally, the study investigates whether a recursive pathway exists from academic emotions back to SRL. Methods The study draws on nationwide survey data from China ( N = 88,149 students) and employs structural equation modeling (SEM) to analyze the relationships among SRL, academic emotions, TSR, and academic achievement. Academic emotions were included as a mediating variable, and TSR as a moderating variable. Results The results indicate that: (1) adolescents’ levels of SRL are significantly and positively associated with their academic achievement; (2) three types of academic emotions (e.g., positive high-arousal emotions) significantly mediate the relationship between SRL and academic achievement; and (3) TSR moderate both the first stage of the mediation pathway (“SRL → academic emotions → academic achievement”) and the direct effect of SRL on academic achievement. Discussion Overall, the findings support the cognition–emotion cyclical model, suggesting that students can enhance SRL through positive academic emotions, while appropriate SRL strategies can in turn foster positive academic emotions, forming a virtuous cycle that strengthens students’ autonomy in the learning process. This study extends Pintrich’s SRL model by empirically validating a recursive loop between SRL and academic emotions. Furthermore, it highlights a “dual empowerment” path of emotional regulation and metacognitive monitoring through optimized TSR, offering vital policy insights for fostering high-order autonomous learning in the AI era.
Sun et al. (Tue,) studied this question.