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A Monte Carlo method for calculating quantum mechanical time correlation functions is presented. In this method the time correlation function is calculated at several values along the pure imaginary axis of the complex time plane such that 0itβ, where (β)−1 is the temperature of the system. Using the periodicity of the imaginary time correlation function, the real time behavior is inferred by analytic continuation. The method is used to calculate the absorption spectra of two model systems.
Thirumalai et al. (Tue,) studied this question.