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July 21, 2025Chemical Reviews45 citationsOpen Access

Intelligent Photodetectors: Postmanufacturing Tunability toward Enhanced Performance and Advanced Functions

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YLYuanzhe LiXHXie HeSCShih‐Chi Chen

Key Points

  • Intelligent photodetectors can adjust performance metrics in real-time, enhancing their effectiveness.
  • Postmanufacturing tunability allows for improved spectral response and dynamic range in diverse applications.
  • The review covers foundational principles and innovations in tunable photodetector mechanisms and functionalities.
  • Challenges in current technologies and future opportunities for innovation are discussed, emphasizing adaptive systems.

Abstract

Photodetectors have become essential in modern technologies, yet traditional designs face challenges in many emerging applications owing to their fixed response characteristics, such as fixed responsivity, bandwidth, dynamic range, and spectral response. This limitation reduces their effectiveness when the target signal or ambient light varies in intensity, frequency, and wavelength, etc. Intelligent photodetectors, featuring postmanufacturing tunability, have emerged as a promising solution by allowing for real-time adaptability. These dynamic devices can adjust key performance metrics during operation, enhancing their versatility and applicability. Beyond basic photodetection, this adaptability lays fundamentals for various new functions, for instance, in-sensor computing and computational spectrum reconstruction. Some devices also offer switchable operation modes and integrated multisensory perception, minimizing the need for auxiliary components and simplifying the system architecture. This review aims to provide a comprehensive and holistic view of the diverse advances in intelligent photodetectors under the concept of tunable mechanisms. Beginning with foundational principles, we explore how postmanufacturing tunability enhances basic photodetection performance and enables advanced functions through tunable temporal response dynamics, spectral response, and multiple operational modes. We conclude with challenges and future opportunities, aiming to inspire continued innovation by bridging diverse fields of photodetection through the lens of postmanufacturing tunability.

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Cite This Study

Li et al. (2025) studied this question.

synapsesocial.com/papers/689a060ee6551bb0af8cd36chttps://doi.org/10.1021/acs.chemrev.4c00763
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