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May 23, 2024Nature Communications95 citationsOpen Access

Orbital-dependent electron correlation in double-layer nickelate La3Ni2O7

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JYJiangang YangHSHualei SunXHXunwu Hu

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Abstract

Abstract The latest discovery of high temperature superconductivity near 80 K in La 3 Ni 2 O 7 under high pressure has attracted much attention. Many proposals are put forth to understand the origin of superconductivity. The determination of electronic structures is a prerequisite to establish theories to understand superconductivity in nickelates but is still lacking. Here we report our direct measurement of the electronic structures of La 3 Ni 2 O 7 by high-resolution angle-resolved photoemission spectroscopy. The Fermi surface and band structures of La 3 Ni 2 O 7 are observed and compared with the band structure calculations. Strong electron correlations are revealed which are orbital- and momentum-dependent. A flat band is formed from the Ni-3d ₙ^{2} z2 orbitals around the zone corner which is ~ 50 meV below the Fermi level and exhibits the strongest electron correlation. In many theoretical proposals, this band is expected to play the dominant role in generating superconductivity in La 3 Ni 2 O 7. Our observations provide key experimental information to understand the electronic structure and origin of high temperature superconductivity in La 3 Ni 2 O 7.

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Cite This Study

Yang et al. (2024) studied this question.

synapsesocial.com/papers/68e68ab2b6db64358761280ahttps://doi.org/10.1038/s41467-024-48701-7
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