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April 29, 2026Small0 citations

In Situ Surface Reconstruction and Carbon Encapsulation for High‐Performance Pt‐Lean Catalysts beyond Conventional Core–Shell Designs (Small 24/2026)

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JMJiho MinJLJeong Hee LeeKKKeonwoo Ko

Key Points

  • To investigate a new strategy for developing high-performance catalytic structures with reduced platinum usage.
  • In-situ one-step synthesis of Pt–3d alloy nanoparticles
  • Formation of porous carbon shell surrounding the catalysts
  • Assessment of catalyst durability and activity during the oxygen reduction reaction
  • The synthesized catalysts showed enhanced oxygen reduction activity compared to conventional designs.
  • Catalysts maintained long-term durability with reduced platinum usage.
  • This method offers a practical pathway for developing low-cost, high-performance catalysts.

Abstract

Oxygen Reduction Reaction An in-situ one-step synthesis simultaneously induces Pt surface segregation and forms a porous carbon shell on Pt–3d alloy nanoparticles. The resulting structure stabilizes the catalyst while maintaining high oxygen reduction reaction activity and long-term durability, enabling reduced Pt usage without sacrificing fuel-cell activity. This promising strategy offers a practical pathway toward low-cost, high-performance catalysts beyond conventional core–shell structures. More in the Research Article (e11516), Yun Sik Kang, Joseph T. Hupp, Sung Jong Yoo, Namgee Jung, and co-workers.

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Cite This Study

Min et al. (2026) studied this question.

synapsesocial.com/papers/69f19ff5edf4b46824806a3dhttps://doi.org/10.1002/smll.73116
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Also Consider

Synapse has enriched 5 closely related papers on similar clinical questions. Consider them for comparative context:

  1. 1In Situ Surface Reconstruction and Carbon Encapsulation for High‐Performance Pt‐Lean Catalysts beyond Conventional Core–Shell Designs2026
  2. 2Synthesis and Performance Evaluation of Pt–M Fine Nanoparticles on High‐Surface‐Area Carbon Support for Enhanced Oxygen Reduction Reaction Activity in PEFC2025
  3. 3Engineering a Porous PtCo Catalyst Layer via Multilayer Sputtering and Acid Leaching for Enhanced Oxygen Reduction Reaction2026
  4. 4Self-Assembly Intermetallic PtCu<sub>3</sub> Core with High-Index Faceted Pt Shell for High-Efficiency Oxygen Reduction2024 · 56 citations
  5. 5Hierarchical low Pt-loading “core-shell” electrocatalysts for the oxygen reduction reaction in fuel cells2026 · 1 citations