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May 6, 2026Journal of Materials Chemistry A0 citations

Trifunctional Cobalt Single-Atom Catalyst with Axial Chloride Coordination to Achieve Efficient Methylamine Electrosynthesis: A Constant-Potential DFT Study

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AYAo YangCZChangyan ZhuYCYun‐Jie Chu

Key Points

  • Investigate the efficiency of a cobalt single-atom catalyst for methylamine electrosynthesis.
  • Constant-potential density functional theory (DFT) study
  • Focus on electrochemical reaction pathways
  • Assessment of axial chloride coordination effects
  • Efficient methylamine production demonstrated
  • Nitrate and carbon dioxide effectively utilized for synthesis
  • C-N bond formation rates improved

Abstract

Electrochemical methylamine (MMA) synthesis from nitrate (NO3-) and carbon dioxide (CO2) offers a promising approach for sustainable MMA production, yet its progress remains largely limited due to the sluggish C-N...

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Cite This Study

Yang et al. (2026) studied this question.

synapsesocial.com/papers/69fa980604f884e66b531e8ehttps://doi.org/10.1039/d6ta01804a
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