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May 6, 2026AIChE Journal0 citations

Process intensification of solid‐sorbent DAC via a rotating vortex reactor

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AKAfroditi KourouSCSiyuan ChenBWBing Wang

Key Points

  • To investigate the performance of a rotating vortex reactor for direct air capture and process intensification.
  • Tested adsorption and desorption under different gas velocities and rotation speeds.
  • Examined the bed regimes under centrifugal force conditions and vortex flow.
  • Conducted a cyclic cut-off analysis to assess energy consumption and productivity.
  • Achieved CO2 capture rates of 7.5–13.5 kgCO2/(m3·h).
  • Enabled rapid desorption in less than 10 minutes with hot-air regeneration.
  • Identified design improvements for reducing energy demand.

Abstract

Abstract This work investigates the performance of the rotating vortex reactor (RVR) as a promising intensified contactor for direct air capture (DAC). Both adsorption and desorption are tested across ranges of superficial gas velocities and rotation speeds, thereby tuning the bed regime—packed or fluidized—under a centrifugal force field (known as a high‐gravity condition) and a vortex flow to enhance mass and heat transfer. A cyclic cut‐off analysis further quantifies the contributions of the main energy consumers and clarifies the trade‐offs between productivity and energy demand. The adsorber achieves high volumetric CO 2 capture rates of 7.5–13.5 kgCO 2 /(m 3 ·h), while hot‐air regeneration enables rapid desorption in <10 min. This proof‐of‐concept study shows RVR's potential for process intensification while identifying areas for further improvement in the unit's design and operation to reduce energy demand for DAC.

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Cite This Study

Kourou et al. (2026) studied this question.

synapsesocial.com/papers/69fa98bd04f884e66b53276chttps://doi.org/10.1002/aic.70421
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