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May 6, 2026Energy Advances1 citationsOpen Access

Solid-state prealkylation of electrode architectures to tune solid electrolyte interphase composition

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AMAmanda L. MusgroveAVAnkit VermaMRMarco-Tulio F. Rodrigues

Key Points

  • This research explores how to improve the electrochemical performance of Si anodes by addressing SEI composition.
  • Investigated solid-state prealkylation techniques for electrode architectures.
  • Analyzed the effects of SEI composition on Lithium-ion battery performance.
  • Identified the role of irreversible Li consumption in the performance limitations of Si anodes.
  • Highlighted the impact of fractures on the solid electrolyte interface formation.

Abstract

Efficient electrochemical cycling of certain Si anodes is limited by irreversible Li consumption to form and continually reform the solid electrolyte interface (SEI) due to Si expansion/contraction and fracture.

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Cite This Study

Musgrove et al. (2026) studied this question.

synapsesocial.com/papers/69faa1eb04f884e66b532b53https://doi.org/10.1039/d6ya00065g
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