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May 17, 2026Physics of Fluids0 citations

Ion transport between two flow regions separated by a porous membrane

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DHDongdong HeChinese University of Hong Kong, ShenzhenHHHuaxiong HuangYork UniversityJWJonathan J. WylieCity University of Hong Kong

Key Points

  • This research aims to understand the interactions of ion transport, osmosis, and fluid flow across a porous membrane under different conditions.
  • Utilized matched asymptotic expansions to derive effective boundary conditions for the system.
  • Analyzed steady-state equations to identify critical stability limits for ion transport.
  • Considered the impact of fixed membrane charges and external electric fields on osmotic fluxes.
  • Electrokinetic effects were found to be negligible compared to osmotic effects for typical membranes.
  • A critical stability limit was identified, where exceeding it causes flow reversal and pressure drop.
  • Enhanced transmembrane ion fluxes were achieved with high-permittivity synthetic membranes, reducing the risk of flow reversal.

Abstract

This study investigates the multiscale coupling of electro-diffusive ion transport, osmosis, and fluid flow between two Stokes-flow regions separated by a thin porous membrane that can contain fixed charges. To bypass the numerical challenges posed by thin Debye layers, we employ matched asymptotic expansions to derive effective boundary conditions that reduce the system to a macroscale model where concentration, potential, and fluid motion on either side of the membrane are fully coupled. Our analysis reveals that electrokinetic effects are significantly weaker than a simple scaling argument suggests, remaining negligible for biological and traditional synthetic membranes where osmotic effects dominate. By solving the steady-state equations, we identify a critical stability limit governed by a dimensionless osmotic parameter. Exceeding this limit triggers a localized pressure drop and flow reversal at the channel inlets. This represents a catastrophic failure for applications like micro-dialysis or renal filtration, as it leads to the ingestion of unfiltered fluid. We show that osmotic fluxes can be further enhanced by membrane fixed charges and external electric fields. We also consider the possibility of utilizing modern high-permittivity synthetic membranes to obtain non-negligible electrokinetic effects. We show that these effects can enhance transmembrane ion fluxes with a much lower risk of triggering flow reversal compared to osmotic enhancement. Our asymptotic reduced model serves as a computationally efficient design tool for optimizing microfluidic devices by establishing links between membrane properties, external potentials, and transport efficiency.

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Cite This Study

He et al. (2026) studied this question.

synapsesocial.com/papers/6a095c147880e6d24efe2153https://doi.org/10.1063/5.0319718
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