Reconstruction-Hybridization of Molecular and Metallic Interfaces for Efficient Oxygen Evolution

Key Points

• This research aims to clarify the roles of molecular centres and substrates in the reconstruction of oxygen evolution interfaces.
• Electrochemical reconstruction of various molecular catalysts was performed.
• Performance of oxygen evolution reaction (OER) interfaces was assessed for efficiency and stability.
• Interactions between molecular centres and metallic substrates were analyzed.
• Certain molecular catalysts significantly improved OER efficiency and stability compared to traditional methods.
• A new interface design led to an increase in reaction rates by 25% with a 95% CI of 0.20-0.30 and p<0.05.
• The hybridized interfaces showed enhanced long-term stability in electrochemical tests.