October 12, 2016

Direct Synthesis of Pyrroles by Dehydrogenative Coupling of Diols and Amines Catalyzed by Cobalt Pincer Complexes

PDProsenjit DawIndian Institute of Science Education and Research Berhampur SCSubrata ChakrabortyIndian Institute of Technology Jodhpur JGJai Anand GargIndian Institute of Technology Madras

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Abstract

Herein, the first example of base-metal-catalyzed dehydrogenative coupling of diols and amines to selectively form functionalized 1,2,5-substituted pyrroles liberating water and hydrogen gas as the sole by-products is presented. The reaction is catalyzed by pincer complexes of earth-abundant cobalt.

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Daw et al. (Wed,) studied this question.

synapsesocial.com/papers/69de84e47ed287395e559732 https://doi.org/https://doi.org/10.1002/anie.201607742

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