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A series of pincer-type complexes of Os and Ru have been synthesized and investigated in catalytic alcohol dehydrogenation. The hydrides OsHCl(CO)HN(C2H4PiPr2)2 and OsH2(CO)HN(C2H4PiPr2)2 possess good air, moisture, and thermal stability and are outstanding versatile dehydrogenation catalysts for primary alcohols for reactions of transfer hydrogenation, dehydrogenative coupling, and amine alkylation.
Bertoli et al. (Mon,) studied this question.
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