Spin-Orbit Torque Emerging from Orbital Textures in Centrosymmetric Materials

We unveil a hitherto concealed spin-orbit torque mechanism driven by orbital degrees of freedom in centrosymmetric two-dimensional transition metal dichalcogenides (focusing on PtSe 2 ). Using first-principles simulations, tight-binding models, and large-scale quantum transport calculations, we show that such a mechanism fundamentally stems from a spatial localization of orbital textures at opposite sides of the material, which imprints their symmetries onto spin-orbit coupling effects, further producing efficient and tunable spin-orbit torque. Our study suggests that orbital-spin entanglement at play in centrosymmetric materials can be harnessed as a resource for outperforming conventional spin-orbit torques generated by the Rashba-type effects.