Spectroscopic studies reveal zero-field-splitting in Co II complex, highlighting potential for single-ion magnet applications.
High-spin Co II complex (PPh 4 ) 2 [Co(N 3 ) 4 ] ( Co-N 3 ) has been investigated using advanced spectroscopic techniques [far-IR magneto-spectroscopy (FIRMS), high-frequency and -field EPR (HFEPR), and inelastic neutron scattering (INS)] to study its zero-field-splitting (ZFS),...
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Hand et al. (2025) studied this question.
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