Phosphorylation of nitrogen-doped carbon stabilizes Rh clusters for selective hydroformylation of alkenes to linear aldehydes

Dongrun Wang; Chuang Liu; Guiqin Yu; Suxia Liang; Jiantai Ma; Zhengping Dong

doi:10.1039/d5cy00873e

January 1, 2025Catalysis Science & Technology

Phosphorylation of nitrogen-doped carbon stabilizes Rh clusters for selective hydroformylation of alkenes to linear aldehydes

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Key Points

Phosphorylation significantly improves the stability of Rh clusters, leading to better catalytic performance.
The method increased selectivity toward linear aldehydes in hydroformylation, addressing industry challenges.
Using nitrogen-doped carbon as a support material enhances the efficiency of the hydroformylation process.
This advancement may revolutionize industrial applications involving the production of high-value aldehydes.

Implication

Phosphorylation enhances catalyst stability, improving hydroformylation selectivity for linear aldehydes.

Abstract

Hydroformylation of olefins to produce high-value aldehydes is among the most important processes in the chemical industry. However, heterogeneous hydroformylation catalysts still face major challenges, including limited selectivity toward linear...

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Cite This Study

Wang et al. (2025) studied this question.

synapsesocial.com/papers/68c183fe9b7b07f3a06100fa https://doi.org/10.1039/d5cy00873e

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Phosphorylation of nitrogen-doped carbon stabilizes Rh clusters for selective hydroformylation of alkenes to linear aldehydes

Key Points

Implication

Abstract

Discussion

Cite This Study

Phosphorylation of nitrogen-doped carbon stabilizes Rh clusters for selective hydroformylation of alkenes to linear aldehydes

Key Points

Implication

Abstract

Discussion

Cite This Study

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