Analysis of the Seebeck coefficient reveals quantum criticality in clean nickelate films, suggesting implications for superconductivity.
We investigate the Seebeck coefficient (S) in infinite-layer nickelate films with different disorder levels. The disordered NdNiO₂ film exhibits a flat $S/T$ curve, whereas cleaner samples display a logarithmic divergence with decreasing temperature, followed by a pronounced ``hump'' near 25 K. These distinct behaviors reveal a disorder-driven transition from band-structure-dominated transport to quantum-critical-dominated transport. Below the ``hump'' temperature, four-fold symmetry breaking is observed in the in-plane angular magnetoresistance, indicating the presence of short-range antiferromagnetic order in parent infinite-layer nickelate films. Furthermore, the logarithmic divergence in $S/T$ is also observed in a clean superconducting Sm0.73Ca0.05Eu0.22NiO₂ film, where it coexists with linear-in-temperature resistivity over the same temperature range. These findings demonstrate the existence of quantum criticality over a wide doping range in clean infinite-layer nickelate films, similar to cuprates, which highlights the central role of antiferromagnetic spin correlations in their superconducting pairing mechanisms.
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Zhang et al. (2025) studied this question.
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