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October 2, 2025ACS Applied Energy Materials2 citationsOpen Access

Origin of High-Rate Performance of Sb2Se3/Sb Composite Anodes for Na-Ion Batteries

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ASAmalie SkurtveitFMFaduma M. MaddarIHIvana Hasa

Key Points

  • The Sb2Se3/Sb composite anodes achieved a reversible capacity of 360 mAh g–1 at 1000 mA g–1, indicating excellent performance.
  • Operando x-ray diffraction revealed synergies in (de)sodiation mechanisms that enhance both capacity and stability of the anodes.
  • Sodiated phases' amorphization promotes rapid Na-diffusion within the composite structure, improving efficiency.
  • This work highlights the necessity for continuous optimization in materials and structure to maximize performance in sodium-ion batteries.

Abstract

Improving the energy density of Na-ion batteries (NIBs) requires advances in anode materials. This study investigates Sb2Se3/Sb composite anodes, which offer better capacity and stability than the individual constituents. Operando X-ray diffraction (XRD) revealed that (de)sodiation is driven by synergies between the operating mechanisms of Sb2Se3 and Sb, enabling a reversible capacity of 360 mAh g–1 (at 1000 mA g–1). This performance is also aided by amorphization of the sodiated phases, which promotes rapid Na-diffusion. The work emphasizes the need for continuous material and structural optimizations to fully harness their benefits for enabling efficient and fast-charging NIBs.

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Cite This Study

Skurtveit et al. (2025) studied this question.

synapsesocial.com/papers/68de796d5b556a9128e1af42https://doi.org/10.1021/acsaem.5c02418
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