Analysis of tetra-coordinated nonheme iron(IV)-oxo complexes reveals geometry-driven epoxidation and hydroxylation reactivity, highlighting structural controls on oxidation catalysis.
The electronic structure and reactivity of tetra-coordinated nonheme iron(IV)-oxo complexes have remained unexplored for years. The recent synthesis of a closed-shell iron(IV)-oxo complex [(quinisox)Fe
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Bhardwaj et al. (2024) studied this question.
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