Charge Transfer Process Surface-specific in situ VSFG spectroscopy elucidated the compositional and electronic evolution of a Co-PBA interfaces during electrochemical oxidation of the material. This is a happy pairing of nonlinear VSFG spectroscopy and electrochemistry. The methodology is applied for the first time to Prussian Blue analogues and reveals structural and oxidation-state information from both the Co-PBA|electrolyte and the Co-PBA|TiO2-electrode interfaces. The findings in article 2400009 by Ferdi Karadaş, Benjamin Dietzek-Ivanšić, and co-workers showcase that the metal sites in the interface undergo different structural changes than the ones in the bulk.
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Bera et al. (2024) studied this question.
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