Topological Weyl Altermagnetism in CrSb

Altermagnets constitute a novel, third fundamental class of collinear magnetic ordered materials, alongside with ferro- and antiferromagnets. They share with conventional antiferromagnets the feature of a vanishing net magnetization. At the same time they show a spin-splitting of electronic bands, just as in ferromagnets, caused by the atomic exchange interaction. Interestingly, the altermagnetic spin-splitting may in principle allow for topological electronic structures far beyond collinear antiferromagnets with spin-degenerate bands. Here, using high-resolution and spin angle-resolved photoemission spectroscopy, we observe that the momentum-dependent spin-splitting in altermagnetic CrSb reaches up to 1 eV, while vanishing at high symmetry lines in the Brillouin zone. We find it causes spin-carrying altermagnetic Weyl points, and observe their protected Fermi-arc surface states. This establishes that in altermagnets the large energy scale intrinsic to the spin-splitting - orders of magnitude larger that the relativistic spin-orbit coupling - creates its own realm of robust electronic topology, with spin-polarized topological surface states that are altermagnetic.