Probing H2 Double Ionization with Bicircular Laser Fields

We present a kinematically complete study on strong-field double ionization of H₂ molecules in two-color bicircular laser fields. The releasing times of electrons and protons are recorded with the double-hand attoclock. We observe the relative emission angles of two electrons oscillate with the kinetic energy release of protons, indicating the internal concerted four-body fragmentation. Using a three-dimensional molecular semiclassical ensemble model, we have disentangled the attosecond correlated electron emission in H₂ double ionization. This work reveals the strong electron-nuclear coupling in the molecular bond breaking and may open up a new approach to experimentally accessing the intramolecular electron and bond dynamics with bicircular fields.